Colossal magnetocapacitance and scale-invariant dielectric response in phase-separated manganites

Ryan P. Rairigh, Guneeta Singh-Bhalla, Sefaattin Tongay, Tara Dhakal, Amlan Biswas, Arthur F. Hebard

Research output: Contribution to journalArticle

42 Citations (Scopus)

Abstract

Afull characterization of phase separation and the competition between phases is necessary for a comprehensive understanding of strongly correlated electron materials, such as under-doped high-temperature superconductors, complex oxide heterojunctions, spinels, multiferroics, rare-earth ferroelectric manganites and mixed-valence manganites in which phase competition is the dominant mechanism governing the insulator-metal (IM) transition and the associated colossal magnetoresistance effect. Thin films of strongly correlated electron materials are often grown epitaxially on planar substrates and typically have anisotropic properties that are usually not captured by edge-mounted four-terminal electrical measurements, which are primarily sensitive to in-plane conduction paths. We present an experimental study of anisotropic transport in phase-separated manganite thin films by using an unconventional arrangement of contact electrodes that enables the simultaneous determination of colossal magnetoresistance associated with d.c. transport parallel to the film substrate and colossal magnetocapacitance associated with a.c. transport in the perpendicular direction. We distinguish two distinct direction-dependent IM transitions and find a dielectric response that collapses onto a scale-invariant dependence over a large range of frequency, temperature and magnetic field.

Original languageEnglish (US)
Pages (from-to)551-555
Number of pages5
JournalNature Physics
Volume3
Issue number8
DOIs
StatePublished - Aug 2007
Externally publishedYes

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transition metals
insulators
thin films
high temperature superconductors
electrical measurement
heterojunctions
temperature distribution
electrons
rare earth elements
valence
conduction
electrodes
oxides
magnetic fields

ASJC Scopus subject areas

  • Physics and Astronomy(all)

Cite this

Colossal magnetocapacitance and scale-invariant dielectric response in phase-separated manganites. / Rairigh, Ryan P.; Singh-Bhalla, Guneeta; Tongay, Sefaattin; Dhakal, Tara; Biswas, Amlan; Hebard, Arthur F.

In: Nature Physics, Vol. 3, No. 8, 08.2007, p. 551-555.

Research output: Contribution to journalArticle

Rairigh, RP, Singh-Bhalla, G, Tongay, S, Dhakal, T, Biswas, A & Hebard, AF 2007, 'Colossal magnetocapacitance and scale-invariant dielectric response in phase-separated manganites', Nature Physics, vol. 3, no. 8, pp. 551-555. https://doi.org/10.1038/nphys626
Rairigh, Ryan P. ; Singh-Bhalla, Guneeta ; Tongay, Sefaattin ; Dhakal, Tara ; Biswas, Amlan ; Hebard, Arthur F. / Colossal magnetocapacitance and scale-invariant dielectric response in phase-separated manganites. In: Nature Physics. 2007 ; Vol. 3, No. 8. pp. 551-555.
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