Anomalous carrier dynamics and localization effects in nonpolar m-plane InGaN/GaN quantum wells at high temperatures

Xuanqi Huang, Dongying Li, Po Yi Su, Houqiang Fu, Hong Chen, Chen Yang, Jingan Zhou, Xin Qi, Tsung Han Yang, Jossue Montes, Xuguang Deng, Kai Fu, Steven P. DenBaars, Shuji Nakamura, Fernando A. Ponce, Cun Zheng Ning, Yuji Zhao

Research output: Contribution to journalArticle

Abstract

Nonpolar InGaN/GaN quantum wells (QWs) have gained significance for efficient light emitting since it eliminates polarization-related effects and allows for higher radiative capability. Although much progress has been made in analyzing carrier localization effects at cryogenic temperatures, carrier dynamics at above room temperatures are still not well understood. In this work, we have observed and explored anomalous carrier dynamics of two nonpolar m-plane InGaN/GaN QWs at high temperatures by combining scanning transmission electron microscopy (STEM) and photophysical characterization. Both experimental and theoretical results suggest that carrier lifetime in both samples increases with temperature in a certain range of temperature. However, the reduced integrity and uniformity of QWs make carriers more prone to the nonradiative Shockley-Reed-Hall recombination as temperature rises. Moreover, both acoustic and optical phonon scatterings dominate from 300 to 600 K through the analysis on the evolution of photoluminescence spectra. Overall, these detailed studies provide insights into approaches to evaluate carrier dynamics at elevated temperatures and improve emitting performance to further push the practical efficiency limit.

Original languageEnglish (US)
Article number105013
JournalNano Energy
Volume76
DOIs
StatePublished - Oct 2020
Externally publishedYes

Keywords

  • Carrier dynamics
  • High temperature
  • InGaN
  • Localization
  • Quantum wells

ASJC Scopus subject areas

  • Renewable Energy, Sustainability and the Environment
  • Materials Science(all)
  • Electrical and Electronic Engineering

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  • Cite this

    Huang, X., Li, D., Su, P. Y., Fu, H., Chen, H., Yang, C., Zhou, J., Qi, X., Yang, T. H., Montes, J., Deng, X., Fu, K., DenBaars, S. P., Nakamura, S., Ponce, F. A., Ning, C. Z., & Zhao, Y. (2020). Anomalous carrier dynamics and localization effects in nonpolar m-plane InGaN/GaN quantum wells at high temperatures. Nano Energy, 76, [105013]. https://doi.org/10.1016/j.nanoen.2020.105013