Wet and dry sizes of atmospheric aerosol particles

An AFM-TEM study

Mihály Pósfai, Huifang Xu, James R. Anderson, P R Buseck

Research output: Contribution to journalArticle

90 Citations (Scopus)

Abstract

We studied the hygroscopic behavior of atmospheric aerosols by using a novel approach, the combination of atomic force microscopy (AFM) with transmission electron microscopy (TEM) imaging of the same individual particles. By comparing the dimensions of hydrated and dry ammonium sulfate particles collected above the North Atlantic Ocean, we determined that particle volumes are up to four times larger under ambient conditions (as determined by AFM) than in the vacuum of a transmission electron microscope. We interpret these changes as resulting from the loss of water. Organic films on the particles may be responsible for the relatively large water uptake at low relative humidities.

Original languageEnglish (US)
Pages (from-to)1907-1910
Number of pages4
JournalGeophysical Research Letters
Volume25
Issue number10
StatePublished - Jun 1 1998

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atomic force microscopy
transmission electron microscopy
aerosols
aerosol
ammonium sulfates
Atlantic Ocean
water uptake
ammonium sulfate
water
humidity
relative humidity
electron microscopes
electron
vacuum
particle

ASJC Scopus subject areas

  • Earth and Planetary Sciences (miscellaneous)

Cite this

Wet and dry sizes of atmospheric aerosol particles : An AFM-TEM study. / Pósfai, Mihály; Xu, Huifang; Anderson, James R.; Buseck, P R.

In: Geophysical Research Letters, Vol. 25, No. 10, 01.06.1998, p. 1907-1910.

Research output: Contribution to journalArticle

Pósfai, M, Xu, H, Anderson, JR & Buseck, PR 1998, 'Wet and dry sizes of atmospheric aerosol particles: An AFM-TEM study', Geophysical Research Letters, vol. 25, no. 10, pp. 1907-1910.
Pósfai, Mihály ; Xu, Huifang ; Anderson, James R. ; Buseck, P R. / Wet and dry sizes of atmospheric aerosol particles : An AFM-TEM study. In: Geophysical Research Letters. 1998 ; Vol. 25, No. 10. pp. 1907-1910.
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