Variability of heterostructure type with thickness of barriers and temperature in the InAs/GaAsSb quantum dot system

A. Pancholi, S. P. Bremner, J. Boyle, V. G. Stoleru, Christiana Honsberg

Research output: Contribution to journalArticle

12 Citations (Scopus)

Abstract

We report photoluminescence studies of InAs quantum dots embedded in GaAsSb barrier layers of various thicknesses. Time resolved photoluminescence results suggest that the thicknesses of the GaAsSb barrier layers determines whether the quantum dot system acts as a type I (thicker) or type II (thinner) heterostructure due to strain induced changes in the band energies. Temperature dependent photoluminescence reveal that the transition type is also dependent on the temperature with one sample seeming to transform from type II to type I heterostructure as the temperature is increased. These results support previous assertions that it is possible to obtain a zero valence band offset in the InAs/GaAsSb quantum dot system, making it a system of interest for realization of a novel photovoltaic structure, the intermediate band solar cell. The results highlight some of the inherent issues in designing structures with specific band offsets. Some of the implications of these results on the design methodology for quantum dot based solar cells are briefly discussed.

Original languageEnglish (US)
Pages (from-to)1025-1030
Number of pages6
JournalSolar Energy Materials and Solar Cells
Volume94
Issue number6
DOIs
StatePublished - Jun 2010
Externally publishedYes

Fingerprint

Semiconductor quantum dots
Heterojunctions
Photoluminescence
Solar cells
Temperature
Valence bands
Band structure
indium arsenide

Keywords

  • Photoluminescence
  • Quantum dot solar cell
  • Type I/II heterostructure

ASJC Scopus subject areas

  • Renewable Energy, Sustainability and the Environment
  • Electronic, Optical and Magnetic Materials
  • Surfaces, Coatings and Films

Cite this

Variability of heterostructure type with thickness of barriers and temperature in the InAs/GaAsSb quantum dot system. / Pancholi, A.; Bremner, S. P.; Boyle, J.; Stoleru, V. G.; Honsberg, Christiana.

In: Solar Energy Materials and Solar Cells, Vol. 94, No. 6, 06.2010, p. 1025-1030.

Research output: Contribution to journalArticle

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AU - Honsberg, Christiana

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