Ultraintense x-ray induced ionization, dissociation, and frustrated absorption in molecular nitrogen

M. Hoener; L. Fang; O. Kornilov; O. Gessner; S. T. Pratt; M. Gühr; E. P. Kanter; C. Blaga; C. Bostedt; J. D. Bozek; P. H. Bucksbaum; C. Buth; M. Chen; R. Coffee; J. Cryan; L. Dimauro; M. Glownia; E. Hosler; E. Kukk; S. R. Leone; B. McFarland; M. Messerschmidt; B. Murphy; V. Petrovic; D. Rolles; N. Berrah

doi:10.1103/PhysRevLett.104.253002

Ultraintense x-ray induced ionization, dissociation, and frustrated absorption in molecular nitrogen

M. Hoener, L. Fang, O. Kornilov, O. Gessner, S. T. Pratt, M. Gühr, E. P. Kanter, C. Blaga, C. Bostedt, J. D. Bozek, P. H. Bucksbaum, C. Buth, M. Chen, R. Coffee, J. Cryan, L. Dimauro, M. Glownia, E. Hosler, E. Kukk, S. R. LeoneB. McFarland, M. Messerschmidt, B. Murphy, V. Petrovic, D. Rolles, N. Berrah

Research output: Contribution to journal › Article › peer-review

178 Scopus citations

Abstract

Sequential multiple photoionization of the prototypical molecule N2 is studied with femtosecond time resolution using the Linac Coherent Light Source (LCLS). A detailed picture of intense x-ray induced ionization and dissociation dynamics is revealed, including a molecular mechanism of frustrated absorption that suppresses the formation of high charge states at short pulse durations. The inverse scaling of the average target charge state with x-ray peak brightness has possible implications for single-pulse imaging applications.

Original language	English (US)
Article number	253002
Journal	Physical Review Letters
Volume	104
Issue number	25
DOIs	https://doi.org/10.1103/PhysRevLett.104.253002
State	Published - Jun 23 2010
Externally published	Yes

ASJC Scopus subject areas

General Physics and Astronomy

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Hoener, M., Fang, L., Kornilov, O., Gessner, O., Pratt, S. T., Gühr, M., Kanter, E. P., Blaga, C., Bostedt, C., Bozek, J. D., Bucksbaum, P. H., Buth, C., Chen, M., Coffee, R., Cryan, J., Dimauro, L., Glownia, M., Hosler, E., Kukk, E., ... Berrah, N. (2010). Ultraintense x-ray induced ionization, dissociation, and frustrated absorption in molecular nitrogen. Physical Review Letters, 104(25), Article 253002. https://doi.org/10.1103/PhysRevLett.104.253002

Hoener, M, Fang, L, Kornilov, O, Gessner, O, Pratt, ST, Gühr, M, Kanter, EP, Blaga, C, Bostedt, C, Bozek, JD, Bucksbaum, PH, Buth, C, Chen, M, Coffee, R, Cryan, J, Dimauro, L, Glownia, M, Hosler, E, Kukk, E, Leone, SR, McFarland, B, Messerschmidt, M, Murphy, B, Petrovic, V, Rolles, D & Berrah, N 2010, 'Ultraintense x-ray induced ionization, dissociation, and frustrated absorption in molecular nitrogen', Physical Review Letters, vol. 104, no. 25, 253002. https://doi.org/10.1103/PhysRevLett.104.253002

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abstract = "Sequential multiple photoionization of the prototypical molecule N2 is studied with femtosecond time resolution using the Linac Coherent Light Source (LCLS). A detailed picture of intense x-ray induced ionization and dissociation dynamics is revealed, including a molecular mechanism of frustrated absorption that suppresses the formation of high charge states at short pulse durations. The inverse scaling of the average target charge state with x-ray peak brightness has possible implications for single-pulse imaging applications.",

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AU - Hoener, M.

AU - Fang, L.

AU - Kornilov, O.

AU - Gessner, O.

AU - Pratt, S. T.

AU - Gühr, M.

AU - Kanter, E. P.

AU - Blaga, C.

AU - Bostedt, C.

AU - Bozek, J. D.

AU - Bucksbaum, P. H.

AU - Buth, C.

AU - Chen, M.

AU - Coffee, R.

AU - Cryan, J.

AU - Dimauro, L.

AU - Glownia, M.

AU - Hosler, E.

AU - Kukk, E.

AU - Leone, S. R.

AU - McFarland, B.

AU - Messerschmidt, M.

AU - Murphy, B.

AU - Petrovic, V.

AU - Rolles, D.

AU - Berrah, N.

PY - 2010/6/23

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Ultraintense x-ray induced ionization, dissociation, and frustrated absorption in molecular nitrogen

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