Abstract
We give a detailed account of the theoretical analysis and the experimental results of an X-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric rotor molecule 2,5-diiodobenzonitrile, performed at the Linac Coherent Light Source [Phys. Rev. Lett. 112, 083002 (2014)]. This experiment is the first step toward coherent diffractive imaging of structures and structural dynamics of isolated molecules at atomic resolution, i.e., picometers and femtoseconds, using X-ray free-electron lasers.
| Original language | English (US) |
|---|---|
| Pages (from-to) | 393-418 |
| Number of pages | 26 |
| Journal | Faraday Discussions |
| Volume | 171 |
| DOIs | |
| State | Published - Jan 1 2014 |
| Externally published | Yes |
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ASJC Scopus subject areas
- Physical and Theoretical Chemistry
Cite this
Toward atomic resolution diffractive imaging of isolated molecules with X-ray free-electron lasers. / Stern, S.; Holmegaard, L.; Filsinger, F.; Rouzée, A.; Rudenko, A.; Johnsson, P.; Martin, A. V.; Barty, A.; Bostedt, C.; Bozek, J.; Coffee, R.; Epp, S.; Erk, B.; Foucar, L.; Hartmann, R.; Kimmel, N.; Kühnel, K. U.; Maurer, J.; Messerschmidt, Marc; Rudek, B.; Starodub, D.; Thøgersen, J.; Weidenspointner, G.; White, T. A.; Stapelfeldt, H.; Rolles, D.; Chapman, H. N.; Küpper, J.
In: Faraday Discussions, Vol. 171, 01.01.2014, p. 393-418.Research output: Contribution to journal › Article
}
TY - JOUR
T1 - Toward atomic resolution diffractive imaging of isolated molecules with X-ray free-electron lasers
AU - Stern, S.
AU - Holmegaard, L.
AU - Filsinger, F.
AU - Rouzée, A.
AU - Rudenko, A.
AU - Johnsson, P.
AU - Martin, A. V.
AU - Barty, A.
AU - Bostedt, C.
AU - Bozek, J.
AU - Coffee, R.
AU - Epp, S.
AU - Erk, B.
AU - Foucar, L.
AU - Hartmann, R.
AU - Kimmel, N.
AU - Kühnel, K. U.
AU - Maurer, J.
AU - Messerschmidt, Marc
AU - Rudek, B.
AU - Starodub, D.
AU - Thøgersen, J.
AU - Weidenspointner, G.
AU - White, T. A.
AU - Stapelfeldt, H.
AU - Rolles, D.
AU - Chapman, H. N.
AU - Küpper, J.
PY - 2014/1/1
Y1 - 2014/1/1
N2 - We give a detailed account of the theoretical analysis and the experimental results of an X-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric rotor molecule 2,5-diiodobenzonitrile, performed at the Linac Coherent Light Source [Phys. Rev. Lett. 112, 083002 (2014)]. This experiment is the first step toward coherent diffractive imaging of structures and structural dynamics of isolated molecules at atomic resolution, i.e., picometers and femtoseconds, using X-ray free-electron lasers.
AB - We give a detailed account of the theoretical analysis and the experimental results of an X-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric rotor molecule 2,5-diiodobenzonitrile, performed at the Linac Coherent Light Source [Phys. Rev. Lett. 112, 083002 (2014)]. This experiment is the first step toward coherent diffractive imaging of structures and structural dynamics of isolated molecules at atomic resolution, i.e., picometers and femtoseconds, using X-ray free-electron lasers.
UR - http://www.scopus.com/inward/record.url?scp=84911992515&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=84911992515&partnerID=8YFLogxK
U2 - 10.1039/c4fd00028e
DO - 10.1039/c4fd00028e
M3 - Article
VL - 171
SP - 393
EP - 418
JO - Faraday Discussions
JF - Faraday Discussions
SN - 1364-5498
ER -