Subnanosecond phase transition dynamics in laser-shocked iron

H. Hwang, E. Galtier, H. Cynn, I. Eom, S. H. Chun, Y. Bang, G. C. Hwang, J. Choi, T. Kim, M. Kong, S. Kwon, K. Kang, H. J. Lee, C. Park, J. I. Lee, Yongmoon Lee, W. Yang, S. H. Shim, T. Vogt, Sangsoo KimJ. Park, Sunam Kim, D. Nam, J. H. Lee, H. Hyun, M. Kim, T. Y. Koo, C. C. Kao, T. Sekine, T. Sekine, Yongjae Lee, Yongjae Lee

Research output: Contribution to journalArticle

Abstract

Iron is one of the most studied chemical elements due to its sociotechnological and planetary importance; hence, understanding its structural transition dynamics is of vital interest. By combining a short pulse optical laser and an ultrashort free electron laser pulse, we have observed the subnanosecond structural dynamics of iron from high-quality x-ray diffraction data measured at 50-ps intervals up to 2500 ps. We unequivocally identify a threewave structure during the initial compression and a two-wave structure during the decaying shock, involving all of the known structural types of iron (α-, γ-, and ϵ-phase). In the final stage, negative lattice pressures are generated by the propagation of rarefaction waves, leading to the formation of expanded phases and the recovery of γ-phase. Our observations demonstrate the unique capability of measuring the atomistic evolution during the entire lattice compression and release processes at unprecedented time and strain rate.

Original languageEnglish (US)
Article numberEAAZ5132
JournalScience Advances
Volume6
Issue number23
DOIs
StatePublished - Jun 2020

ASJC Scopus subject areas

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    Hwang, H., Galtier, E., Cynn, H., Eom, I., Chun, S. H., Bang, Y., Hwang, G. C., Choi, J., Kim, T., Kong, M., Kwon, S., Kang, K., Lee, H. J., Park, C., Lee, J. I., Lee, Y., Yang, W., Shim, S. H., Vogt, T., ... Lee, Y. (2020). Subnanosecond phase transition dynamics in laser-shocked iron. Science Advances, 6(23), [EAAZ5132]. https://doi.org/10.1126/sciadv.aaz5132