State-resolved attosecond reversible and irreversible dynamics in strong optical fields

Mazyar Sabbar, Henry Timmers, Yi Jen Chen, Allison K. Pymer, Zhi Heng Loh, Scott Sayres, Stefan Pabst, Robin Santra, Stephen R. Leone

Research output: Contribution to journalArticle

24 Citations (Scopus)

Abstract

Strong-field ionization (SFI) is a key process for accessing real-time quantum dynamics of electrons on the attosecond timescale. The theoretical foundation of SFI was pioneered in the 1960s, and later refined by various analytical models. While asymptotic ionization rates predicted by these models have been tested to be in reasonable agreement for a wide range of laser parameters, predictions for SFI on the sub-laser-cycle timescale are either beyond the scope of the models or show strong qualitative deviations from full quantum-mechanical simulations. Here, using the unprecedented state specificity of attosecond transient absorption spectroscopy, we follow the real-time SFI process of the two valence spin-orbit states of xenon. The results reveal that the irreversible tunnelling contribution is accompanied by a reversible electronic population that exhibits an observable spin-orbit-dependent phase delay. A detailed theoretical analysis attributes this observation to transient ground-state polarization, an unexpected facet of SFI that cannot be captured by existing analytical models that focus exclusively on the production of asymptotic electron/ion yields.

Original languageEnglish (US)
Pages (from-to)472-478
Number of pages7
JournalNature Physics
Volume13
Issue number5
DOIs
StatePublished - May 3 2017

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ionization
orbits
xenon
lasers
flat surfaces
absorption spectroscopy
electrons
valence
deviation
cycles
ground state
polarization
predictions
electronics
ions
simulation

ASJC Scopus subject areas

  • Physics and Astronomy(all)

Cite this

Sabbar, M., Timmers, H., Chen, Y. J., Pymer, A. K., Loh, Z. H., Sayres, S., ... Leone, S. R. (2017). State-resolved attosecond reversible and irreversible dynamics in strong optical fields. Nature Physics, 13(5), 472-478. https://doi.org/10.1038/nphys4027

State-resolved attosecond reversible and irreversible dynamics in strong optical fields. / Sabbar, Mazyar; Timmers, Henry; Chen, Yi Jen; Pymer, Allison K.; Loh, Zhi Heng; Sayres, Scott; Pabst, Stefan; Santra, Robin; Leone, Stephen R.

In: Nature Physics, Vol. 13, No. 5, 03.05.2017, p. 472-478.

Research output: Contribution to journalArticle

Sabbar, M, Timmers, H, Chen, YJ, Pymer, AK, Loh, ZH, Sayres, S, Pabst, S, Santra, R & Leone, SR 2017, 'State-resolved attosecond reversible and irreversible dynamics in strong optical fields', Nature Physics, vol. 13, no. 5, pp. 472-478. https://doi.org/10.1038/nphys4027
Sabbar, Mazyar ; Timmers, Henry ; Chen, Yi Jen ; Pymer, Allison K. ; Loh, Zhi Heng ; Sayres, Scott ; Pabst, Stefan ; Santra, Robin ; Leone, Stephen R. / State-resolved attosecond reversible and irreversible dynamics in strong optical fields. In: Nature Physics. 2017 ; Vol. 13, No. 5. pp. 472-478.
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