Real-time coarsening dynamics of Ge/Si(100) nanostructures using elevated temperature scanning tunneling microscopy

Michael R. Mckay, Jeffery Drucker, John Shumway

Research output: Chapter in Book/Report/Conference proceedingConference contribution

Abstract

Coarsening dynamics of Ge/Si(100) nanostructures were monitored using real-time, elevated temperature scanning tunneling microscopy. Gas-source molecular beam epitaxy from digermane at 0.2 ML / min onto Si(100) at temperatures near 500°C produced mixed hut and pyramid cluster ensembles. The width of the most elongated rectangular-based hut clusters is always less than the side length of square-based pyramid clusters for island ensembles grown using these conditions. This suggests that pyramid elongation to form hut clusters occurred at early growth stages for some smaller clusters. Growth temperature annealing revealed that pyramid clusters are more stable than narrow hut clusters with larger volumes, These larger volume huts decay by reducing their length at constant width, finally becoming small pyramids. These pyramids, which are smaller than those which never elongated to form huts, are less stable and consequently dissolve. Atomistic elastic modeling confirms that hut clusters less efficiently store elastic energy than pyramid clusters which explains our observations, Large (> 1μm diameter), low chemical potential clusters deplete the surface of Ge adatoms as evidenced by the existence of denuded zones devoid of smaller clusters. These large clusters are responsible for the decrease in total island volume in the STM field of view during the anneal.

Original languageEnglish (US)
Title of host publicationStability of Thin Films and Nanostructures
Pages52-57
Number of pages6
StatePublished - Dec 1 2004
Event2004 MRS Fall Meeting - Boston, MA, United States
Duration: Nov 29 2004Dec 3 2004

Publication series

NameMaterials Research Society Symposium Proceedings
Volume854
ISSN (Print)0272-9172

Other

Other2004 MRS Fall Meeting
CountryUnited States
CityBoston, MA
Period11/29/0412/3/04

ASJC Scopus subject areas

  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanics of Materials
  • Mechanical Engineering

Fingerprint Dive into the research topics of 'Real-time coarsening dynamics of Ge/Si(100) nanostructures using elevated temperature scanning tunneling microscopy'. Together they form a unique fingerprint.

  • Cite this

    Mckay, M. R., Drucker, J., & Shumway, J. (2004). Real-time coarsening dynamics of Ge/Si(100) nanostructures using elevated temperature scanning tunneling microscopy. In Stability of Thin Films and Nanostructures (pp. 52-57). (Materials Research Society Symposium Proceedings; Vol. 854).