Parity-forbidden excitations of Sr2CuO2Cl2 revealed by optical third-harmonic spectroscopy

A. B. Schumacher; J. S. Dodge; M. A. Carnahan; R. A. Kaindl; D. S. Chemla; L. L. Miller

Parity-forbidden excitations of Sr₂CuO₂Cl₂ revealed by optical third-harmonic spectroscopy

A. B. Schumacher, J. S. Dodge, M. A. Carnahan, R. A. Kaindl, D. S. Chemla, L. L. Miller

Research output: Contribution to journal › Article › peer-review

Abstract

The symmetry and spectrum of both even and odd-parity states near the charge-transfer gap of Sr₂CuO₂Cl₂ were taken into account using nonlinear optical spectroscopy. Polarization analysis of the nonlinear optical response provided evidence for an even-parity state at 2 eV, with a_1g symmetry, and allowed to estimate the magnitude of the dipole matrix element that couples this excitation to the CT exciton.

Original language	English (US)
Article number	127006
Pages (from-to)	127006/1-127006/4
Journal	Physical Review Letters
Volume	87
Issue number	12
State	Published - Sep 17 2001
Externally published	Yes

ASJC Scopus subject areas

General Physics and Astronomy

Cite this

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title = "Parity-forbidden excitations of Sr2CuO2Cl2 revealed by optical third-harmonic spectroscopy",

abstract = "The symmetry and spectrum of both even and odd-parity states near the charge-transfer gap of Sr2CuO2Cl2 were taken into account using nonlinear optical spectroscopy. Polarization analysis of the nonlinear optical response provided evidence for an even-parity state at 2 eV, with a1g symmetry, and allowed to estimate the magnitude of the dipole matrix element that couples this excitation to the CT exciton.",

author = "Schumacher, {A. B.} and Dodge, {J. S.} and Carnahan, {M. A.} and Kaindl, {R. A.} and Chemla, {D. S.} and Miller, {L. L.}",

year = "2001",

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language = "English (US)",

volume = "87",

pages = "127006/1--127006/4",

journal = "Physical Review Letters",

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T1 - Parity-forbidden excitations of Sr2CuO2Cl2 revealed by optical third-harmonic spectroscopy

AU - Schumacher, A. B.

AU - Dodge, J. S.

AU - Carnahan, M. A.

AU - Kaindl, R. A.

AU - Chemla, D. S.

AU - Miller, L. L.

PY - 2001/9/17

Y1 - 2001/9/17

N2 - The symmetry and spectrum of both even and odd-parity states near the charge-transfer gap of Sr2CuO2Cl2 were taken into account using nonlinear optical spectroscopy. Polarization analysis of the nonlinear optical response provided evidence for an even-parity state at 2 eV, with a1g symmetry, and allowed to estimate the magnitude of the dipole matrix element that couples this excitation to the CT exciton.

AB - The symmetry and spectrum of both even and odd-parity states near the charge-transfer gap of Sr2CuO2Cl2 were taken into account using nonlinear optical spectroscopy. Polarization analysis of the nonlinear optical response provided evidence for an even-parity state at 2 eV, with a1g symmetry, and allowed to estimate the magnitude of the dipole matrix element that couples this excitation to the CT exciton.

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M3 - Article

AN - SCOPUS:33745759171

SN - 0031-9007

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JO - Physical Review Letters

JF - Physical Review Letters

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ER -

Parity-forbidden excitations of Sr₂CuO₂Cl₂ revealed by optical third-harmonic spectroscopy

Abstract

ASJC Scopus subject areas

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