Near-unity light absorption in a monolayer ws2 van der waals heterostructure cavity

Itai Epstein, Bernat Terrés, André J. Chaves, Varun Varma Pusapati, Daniel A. Rhodes, Bettina Frank, Valentin Zimmermann, Ying Qin, Kenji Watanabe, Takashi Taniguchi, Harald Giessen, Sefaattin Tongay, James C. Hone, Nuno M.R. Peres, Frank H.L. Koppens

Research output: Contribution to journalArticlepeer-review

11 Scopus citations

Abstract

Excitons in monolayer transition-metal-dichalcogenides (TMDs) dominate their optical response and exhibit strong light-matter interactions with lifetime-limited emission. While various approaches have been applied to enhance light-exciton interactions in TMDs, the achieved strength have been far below unity, and a complete picture of its underlying physical mechanisms and fundamental limits has not been provided. Here, we introduce a TMD-based van der Waals heterostructure cavity that provides near-unity excitonic absorption, and emission of excitonic complexes that are observed at ultralow excitation powers. Our results are in full agreement with a quantum theoretical framework introduced to describe the light-exciton-cavity interaction. We find that the subtle interplay between the radiative, nonradiative and dephasing decay rates plays a crucial role, and unveil a universal absorption law for excitons in 2D systems. This enhanced light-exciton interaction provides a platform for studying excitonic phase-transitions and quantum nonlinearities and enables new possibilities for 2D semiconductor-based optoelectronic devices.

Original languageEnglish (US)
Pages (from-to)3545-3552
Number of pages8
JournalNano Letters
Volume20
Issue number5
DOIs
StatePublished - May 13 2020

Keywords

  • 2D materials
  • Exciton complexes
  • Light-matter interaction
  • TMD Excitons
  • Unity absorption

ASJC Scopus subject areas

  • Bioengineering
  • Chemistry(all)
  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanical Engineering

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