Modeling quantum yield, emittance, and surface roughness effects from metallic photocathodes

D. A. Dimitrov, G. I. Bell, J. Smedley, I. Ben-Zvi, J. Feng, S. Karkare, H. A. Padmore

Research output: Contribution to journalArticle

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Abstract

Detailed measurements of momentum distributions of emitted electrons have allowed the investigation of the thermal limit of the transverse emittance from metal photocathodes. Furthermore, recent developments in material design and growth have resulted in photocathodes that can deliver high quantum efficiency and are sufficiently robust to use in high electric field gradient photoinjectors and free electron lasers. The growth process usually produces photoemissive material layers with rough surface profiles that lead to transverse accelerating fields and possible work function variations, resulting in emittance growth. To better understand the effects of temperature, density of states, and surface roughness on the properties of emitted electrons, we have developed realistic three-dimensional models for photocathode materials with grated surface structures. They include general modeling of electron excitation due to photon absorption, charge transport, and emission from flat and rough metallic surfaces. The models also include image charge and field enhancement effects. We report results from simulations with flat and rough surfaces to investigate how electron scattering, controlled roughness, work function variation, and field enhancement affect emission properties. Comparison of simulation results with measurements of the quantum yield and transverse emittance from flat Sb emission surfaces shows the importance of including efficient modeling of photon absorption, temperature effects, and the material density of states to achieve agreement with the experimental data.

Original languageEnglish (US)
Article number165303
JournalJournal of Applied Physics
Volume122
Issue number16
DOIs
StatePublished - Oct 28 2017
Externally publishedYes

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surface roughness effects
photocathodes
emittance
roughness
electrons
augmentation
photons
three dimensional models
free electron lasers
temperature effects
quantum efficiency
flat surfaces
surface roughness
electron scattering
simulation
momentum
gradients
electric fields
profiles
metals

ASJC Scopus subject areas

  • Physics and Astronomy(all)

Cite this

Dimitrov, D. A., Bell, G. I., Smedley, J., Ben-Zvi, I., Feng, J., Karkare, S., & Padmore, H. A. (2017). Modeling quantum yield, emittance, and surface roughness effects from metallic photocathodes. Journal of Applied Physics, 122(16), [165303]. https://doi.org/10.1063/1.4996568

Modeling quantum yield, emittance, and surface roughness effects from metallic photocathodes. / Dimitrov, D. A.; Bell, G. I.; Smedley, J.; Ben-Zvi, I.; Feng, J.; Karkare, S.; Padmore, H. A.

In: Journal of Applied Physics, Vol. 122, No. 16, 165303, 28.10.2017.

Research output: Contribution to journalArticle

Dimitrov, D. A. ; Bell, G. I. ; Smedley, J. ; Ben-Zvi, I. ; Feng, J. ; Karkare, S. ; Padmore, H. A. / Modeling quantum yield, emittance, and surface roughness effects from metallic photocathodes. In: Journal of Applied Physics. 2017 ; Vol. 122, No. 16.
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