Modeling magneto-optical trapping of CaF molecules

M. R. Tarbutt, Timothy Steimle

Research output: Contribution to journalArticle

23 Citations (Scopus)

Abstract

Magneto-optical trapping forces for molecules are far weaker than for alkali-metal atoms because the photon scattering rate is reduced when there are multiple ground states, and because of optical pumping into dark states. The force is further reduced when the upper state has a much smaller Zeeman splitting than the lower state. We use a rate model to estimate the strength of the trapping and damping forces in a magneto-optical trap (MOT) of CaF molecules, using either the A2Π1/2-X2Σ+ transition or the B2Σ+-X2Σ+ transition. We identify a mechanism of magneto-optical trapping that arises when, in each beam of the MOT, two laser components with opposite polarizations and different detunings address the same transition. This mechanism produces a strong trapping force even when the upper state has little or no Zeeman splitting. It is the main mechanism responsible for the trapping force when the A2Π1/2-X2Σ+ transition is used.

Original languageEnglish (US)
Article number053401
JournalPhysical Review A - Atomic, Molecular, and Optical Physics
Volume92
Issue number5
DOIs
StatePublished - Nov 2 2015

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trapping
molecules
traps
optical pumping
alkali metals
damping
ground state
photons
polarization
estimates
scattering
lasers
atoms

ASJC Scopus subject areas

  • Atomic and Molecular Physics, and Optics

Cite this

Modeling magneto-optical trapping of CaF molecules. / Tarbutt, M. R.; Steimle, Timothy.

In: Physical Review A - Atomic, Molecular, and Optical Physics, Vol. 92, No. 5, 053401, 02.11.2015.

Research output: Contribution to journalArticle

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