TY - JOUR
T1 - Investigation of carrier dynamics in InAs/GaAsSb quantum dots with different silicon delta-doping levels
AU - Ban, Keun Yong
AU - Kim, Yeongho
AU - Kuciauskas, Darius
AU - Bremner, Stephen P.
AU - Honsberg, Christiana
N1 - Funding Information:
This work is in part supported by the National Science Foundation and Department of Energy under Cooperative Agreement No. EEC-1041895.
Publisher Copyright:
© 2016 IOP Publishing Ltd.
PY - 2016/11/10
Y1 - 2016/11/10
N2 - The optical properties of InAs quantum dots (QDs) embedded in a GaAsSb matrix with different delta (δ)-doping levels of 0, 2, 4, and 6 electrons per dot (e-/dot), incorporated to control the occupation of QD electronic states, are studied by photoluminescence (PL) spectroscopy. The time-resolved PL data taken at 10 K reveal that the increase of δ-doping density from 2 to 6 e-/dot decreases the recombination lifetime of carriers at ground states of the QDs from 996 ±36 to 792 ±19 ps, respectively. Furthermore, the carrier lifetime of the sample with 4 e-/dot is found to increase at a slower rate than that of the undoped sample as temperature increases above 70 K. An Arrhenius plot of the temperature dependent PL intensity indicates that the thermal activation energy of electrons in the QDs, required for carrier escape from the dot ground state to continuum state, is increased when the δ-doping density is high enough (>4 e-/dot). These results are attributed to the enhanced Coulomb interaction of electrons provided by the δ-doping, leading to reduced thermal quenching of the PL.
AB - The optical properties of InAs quantum dots (QDs) embedded in a GaAsSb matrix with different delta (δ)-doping levels of 0, 2, 4, and 6 electrons per dot (e-/dot), incorporated to control the occupation of QD electronic states, are studied by photoluminescence (PL) spectroscopy. The time-resolved PL data taken at 10 K reveal that the increase of δ-doping density from 2 to 6 e-/dot decreases the recombination lifetime of carriers at ground states of the QDs from 996 ±36 to 792 ±19 ps, respectively. Furthermore, the carrier lifetime of the sample with 4 e-/dot is found to increase at a slower rate than that of the undoped sample as temperature increases above 70 K. An Arrhenius plot of the temperature dependent PL intensity indicates that the thermal activation energy of electrons in the QDs, required for carrier escape from the dot ground state to continuum state, is increased when the δ-doping density is high enough (>4 e-/dot). These results are attributed to the enhanced Coulomb interaction of electrons provided by the δ-doping, leading to reduced thermal quenching of the PL.
KW - carrier dynamics
KW - delta-doping
KW - intermediate band solar cells
KW - quantum dots
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U2 - 10.1088/0268-1242/31/12/125010
DO - 10.1088/0268-1242/31/12/125010
M3 - Article
AN - SCOPUS:84997079441
SN - 0268-1242
VL - 31
JO - Semiconductor Science and Technology
JF - Semiconductor Science and Technology
IS - 12
M1 - 125010
ER -