Interpretation of dispersive hole-burning kinetics

Research output: Contribution to journalArticle

15 Scopus citations

Abstract

Nonexponential decay of an ensemble of first-order processes are modeled assuming distributions of rate-controlling parameters to be responsible for dispersive kinetics. Some problems of deriving microscopic properties from experimental decay data are illustrated focusing on hole-burning kinetics on the basis of the two-level system model. This approach is compared with reasonings leading to the logarithmic decay law.

Original languageEnglish (US)
Pages (from-to)1743-1747
Number of pages5
JournalThe Journal of chemical physics
Volume86
Issue number4
DOIs
StatePublished - Jan 1 1986

ASJC Scopus subject areas

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

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