Granule formation mechanisms and morphology from single drop impact on powder beds

Heather Emady, Defne Kayrak-Talay, William C. Schwerin, James D. Litster

Research output: Contribution to journalArticle

29 Citations (Scopus)

Abstract

Single drops impacting static powder beds were studied to explain the different resulting granule structures. Three chemically similar powders with different physical properties formed static beds with porosities of 0.66-0.69, 0.54, and 0.30-0.35 respectively. Three different binder fluids (distilled water and silicone oils with viscosities of 9.3 and 96. mPa s) were released onto these powder beds from two different heights (0.5 and 30. cm). The initial drop impact, as well as complete penetration of the droplet into the bed, was recorded with a high speed camera. The high speed camera videos were analyzed, and three different granule formation mechanisms were identified: Tunneling, Spreading, and Crater Formation. Tunneling occurred for loose, cohesive powder beds. Powder aggregates were sucked into the drop which then tunneled into the beds. For coarser powders, granules were formed by a Spreading mechanism at a low impact velocity. At a high impact velocity, the drop formed a crater in the bed surface and deformed elastically in the crater, coating the drop in a layer of powder before penetrating into the bed by capillary action. Using all three dimensions of the granule, a new shape factor, the vertical aspect ratio (the ratio of the granule's projected area diameter to its maximum vertical height), was proposed as a more accurate descriptor of granule shape than currently used descriptors such as the horizontal aspect ratio. The different granule shapes observed were explained by the granule formation mechanisms. The Tunneling mechanism always produced round granules, the Spreading mechanism always produced flat disks, and the Crater Formation mechanism produced granules of varying shapes that were dependant on liquid binder properties. The results of this study have important implications for being able to predict granule structure from granule formation mechanisms, and to be able to choose the desired granule properties by operating in the appropriate regime.

Original languageEnglish (US)
Pages (from-to)69-79
Number of pages11
JournalPowder Technology
Volume212
Issue number1
DOIs
StatePublished - Sep 15 2011
Externally publishedYes

Fingerprint

Powders
High speed cameras
Binders
Aspect ratio
Silicone Oils
Silicones
Physical properties
Porosity
Viscosity
Coatings
Fluids
Water
Liquids

Keywords

  • Crater formation
  • Granule morphology
  • Nucleation
  • Spreading
  • Tunneling
  • Wet granulation

ASJC Scopus subject areas

  • Chemical Engineering(all)

Cite this

Granule formation mechanisms and morphology from single drop impact on powder beds. / Emady, Heather; Kayrak-Talay, Defne; Schwerin, William C.; Litster, James D.

In: Powder Technology, Vol. 212, No. 1, 15.09.2011, p. 69-79.

Research output: Contribution to journalArticle

Emady, Heather ; Kayrak-Talay, Defne ; Schwerin, William C. ; Litster, James D. / Granule formation mechanisms and morphology from single drop impact on powder beds. In: Powder Technology. 2011 ; Vol. 212, No. 1. pp. 69-79.
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