Femtosecond single-shot imaging of nanoscale ferromagnetic order in co/pd multilayers using resonant x-ray holography

Tianhan Wang; Diling Zhu; Benny Wu; Catherine Graves; Stefan Schaffert; Torbjörn Rander; Leonard Müller; Boris Vodungbo; Cédric Baumier; David P. Bernstein; Björn Bräuer; Vincent Cros; Sanne De Jong; Renaud Delaunay; Andreas Fognini; Roopali Kukreja; Sooheyong Lee; Víctor López-Flores; Jyoti Mohanty; Bastian Pfau; Horia Popescu; Maurizio Sacchi; Anna B. Sardinha; Fausto Sirotti; Philippe Zeitoun; Marc Messerschmidt; Joshua J. Turner; William F. Schlotter; Olav Hellwig; Richard Mattana; Nicolas Jaouen; Franck Fortuna; Yves Acremann; Christian Gutt; Hermann A. Dürr; Eric Beaurepaire; Christine Boeglin; Stefan Eisebitt; Gerhard Grübel; Jan Lüning; Joachim Stöhr; Andreas O. Scherz

doi:10.1103/PhysRevLett.108.267403

Femtosecond single-shot imaging of nanoscale ferromagnetic order in co/pd multilayers using resonant x-ray holography

Tianhan Wang, Diling Zhu, Benny Wu, Catherine Graves, Stefan Schaffert, Torbjörn Rander, Leonard Müller, Boris Vodungbo, Cédric Baumier, David P. Bernstein, Björn Bräuer, Vincent Cros, Sanne De Jong, Renaud Delaunay, Andreas Fognini, Roopali Kukreja, Sooheyong Lee, Víctor López-Flores, Jyoti Mohanty, Bastian PfauHoria Popescu, Maurizio Sacchi, Anna B. Sardinha, Fausto Sirotti, Philippe Zeitoun, Marc Messerschmidt, Joshua J. Turner, William F. Schlotter, Olav Hellwig, Richard Mattana, Nicolas Jaouen, Franck Fortuna, Yves Acremann, Christian Gutt, Hermann A. Dürr, Eric Beaurepaire, Christine Boeglin, Stefan Eisebitt, Gerhard Grübel, Jan Lüning, Joachim Stöhr, Andreas O. Scherz

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Abstract

We present the first single-shot images of ferromagnetic, nanoscale spin order taken with femtosecond x-ray pulses. X-ray-induced electron and spin dynamics can be outrun with pulses shorter than 80 fs in the investigated fluence regime, and no permanent aftereffects in the samples are observed below a fluence of 25mJ/cm2. Employing resonant spatially muliplexed x-ray holography results in a low imaging threshold of 5mJ/cm2. Our results open new ways to combine ultrafast laser spectroscopy with sequential snapshot imaging on a single sample, generating a movie of excited state dynamics.

Original language	English (US)
Article number	267403
Journal	Physical Review Letters
Volume	108
Issue number	26
DOIs	https://doi.org/10.1103/PhysRevLett.108.267403
State	Published - Jun 27 2012
Externally published	Yes

ASJC Scopus subject areas

General Physics and Astronomy

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10.1103/PhysRevLett.108.267403

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Wang, T., Zhu, D., Wu, B., Graves, C., Schaffert, S., Rander, T., Müller, L., Vodungbo, B., Baumier, C., Bernstein, D. P., Bräuer, B., Cros, V., De Jong, S., Delaunay, R., Fognini, A., Kukreja, R., Lee, S., López-Flores, V., Mohanty, J., ... Scherz, A. O. (2012). Femtosecond single-shot imaging of nanoscale ferromagnetic order in co/pd multilayers using resonant x-ray holography. Physical Review Letters, 108(26), Article 267403. https://doi.org/10.1103/PhysRevLett.108.267403

Wang, T, Zhu, D, Wu, B, Graves, C, Schaffert, S, Rander, T, Müller, L, Vodungbo, B, Baumier, C, Bernstein, DP, Bräuer, B, Cros, V, De Jong, S, Delaunay, R, Fognini, A, Kukreja, R, Lee, S, López-Flores, V, Mohanty, J, Pfau, B, Popescu, H, Sacchi, M, Sardinha, AB, Sirotti, F, Zeitoun, P, Messerschmidt, M, Turner, JJ, Schlotter, WF, Hellwig, O, Mattana, R, Jaouen, N, Fortuna, F, Acremann, Y, Gutt, C, Dürr, HA, Beaurepaire, E, Boeglin, C, Eisebitt, S, Grübel, G, Lüning, J, Stöhr, J & Scherz, AO 2012, 'Femtosecond single-shot imaging of nanoscale ferromagnetic order in co/pd multilayers using resonant x-ray holography', Physical Review Letters, vol. 108, no. 26, 267403. https://doi.org/10.1103/PhysRevLett.108.267403

@article{212167465eb247d5bad6757e22aa7db3,

title = "Femtosecond single-shot imaging of nanoscale ferromagnetic order in co/pd multilayers using resonant x-ray holography",

abstract = "We present the first single-shot images of ferromagnetic, nanoscale spin order taken with femtosecond x-ray pulses. X-ray-induced electron and spin dynamics can be outrun with pulses shorter than 80 fs in the investigated fluence regime, and no permanent aftereffects in the samples are observed below a fluence of 25mJ/cm2. Employing resonant spatially muliplexed x-ray holography results in a low imaging threshold of 5mJ/cm2. Our results open new ways to combine ultrafast laser spectroscopy with sequential snapshot imaging on a single sample, generating a movie of excited state dynamics.",

author = "Tianhan Wang and Diling Zhu and Benny Wu and Catherine Graves and Stefan Schaffert and Torbj{\"o}rn Rander and Leonard M{\"u}ller and Boris Vodungbo and C{\'e}dric Baumier and Bernstein, {David P.} and Bj{\"o}rn Br{\"a}uer and Vincent Cros and {De Jong}, Sanne and Renaud Delaunay and Andreas Fognini and Roopali Kukreja and Sooheyong Lee and V{\'i}ctor L{\'o}pez-Flores and Jyoti Mohanty and Bastian Pfau and Horia Popescu and Maurizio Sacchi and Sardinha, {Anna B.} and Fausto Sirotti and Philippe Zeitoun and Marc Messerschmidt and Turner, {Joshua J.} and Schlotter, {William F.} and Olav Hellwig and Richard Mattana and Nicolas Jaouen and Franck Fortuna and Yves Acremann and Christian Gutt and D{\"u}rr, {Hermann A.} and Eric Beaurepaire and Christine Boeglin and Stefan Eisebitt and Gerhard Gr{\"u}bel and Jan L{\"u}ning and Joachim St{\"o}hr and Scherz, {Andreas O.}",

note = "Funding Information: We would like to thank I. Ferrero for providing the dIrr data points included in Fig. 4. This work was supported by the Science and Technology Facilities Council [grant number ST/F001166/1 and RF040218], the European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013)/ERC Grant agreement 278594-GasAroundGalaxies, the National Science Foundation under Grant No. PHYS-1066293, the Interuniversity Attraction Poles Programme of the Belgian Science Policy Office [AP P7/08 CHARM] and the hospitality of the Aspen Center for Physics. MF and TS acknowledge the Marie-Curie ITN CosmoComp, and MF also acknowledges the ERC Advanced Grant programme Dustygal. CSF acknowledges an ERC Advanced Investigator Grant COSMIWAY. This work used the DiRAC Data Centric system at Durham University, operated by the Institute for Computational Cosmology on behalf of the STFC DiRAC HPC Facility (www.dirac.ac.uk), and resources provided by WestGrid (www.westgrid.ca) and Compute Canada/Calcul Canada (www.computecanada.ca). The DiRAC system is funded by BIS National E-infrastructure capital grant ST/K00042X/1, STFC capital grant ST/H008519/1, STFC DiRAC Operations grant ST/K003267/1 and Durham University. DiRAC is part of the National E-Infrastructure. Funding Information: We would like to thank I. Ferrero for providing the dIrr data points included in Fig. 4. This work was supported by the Science and Technology Facilities Council [grant number ST/F001166/1 and RF040218], the European Research Council under the European Union{\textquoteright}s Seventh Framework Programme (FP7/2007-2013)/ERC Grant agreement 278594-GasAroundGalaxies, the National Science Foundation under Grant No. PHYS-1066293, the Interuniversity Attraction Poles Programme of the Belgian Science Policy Office [AP P7/08 CHARM] and the hospitality of the Aspen Center for Physics. MF and TS acknowledge the Marie-Curie ITN CosmoComp, and MF also acknowledges the ERC Advanced Grant programme Dustygal. CSF acknowledges an ERC Advanced Investigator Grant COSMIWAY. This work used the DiRAC Data Centric system at Durham University, operated by the Institute for Computational Cosmology on behalf of the STFC DiRAC HPC Facility (www.dirac.ac.uk), and resources provided by WestGrid (www.westgrid.ca) and Compute Canada/Calcul Canada (www.computecanada.ca). The DiRAC system is funded by BIS National E-infrastructure capital grant ST/K00042X/1, STFC capital grant ST/H008519/1, STFC DiRAC Operations grant ST/K003267/1 and Durham University. DiRAC is part of the National E-Infrastructure.",

year = "2012",

month = jun,

day = "27",

doi = "10.1103/PhysRevLett.108.267403",

language = "English (US)",

volume = "108",

journal = "Physical Review Letters",

issn = "0031-9007",

publisher = "American Physical Society",

number = "26",

}

TY - JOUR

T1 - Femtosecond single-shot imaging of nanoscale ferromagnetic order in co/pd multilayers using resonant x-ray holography

AU - Wang, Tianhan

AU - Zhu, Diling

AU - Wu, Benny

AU - Graves, Catherine

AU - Schaffert, Stefan

AU - Rander, Torbjörn

AU - Müller, Leonard

AU - Vodungbo, Boris

AU - Baumier, Cédric

AU - Bernstein, David P.

AU - Bräuer, Björn

AU - Cros, Vincent

AU - De Jong, Sanne

AU - Delaunay, Renaud

AU - Fognini, Andreas

AU - Kukreja, Roopali

AU - Lee, Sooheyong

AU - López-Flores, Víctor

AU - Mohanty, Jyoti

AU - Pfau, Bastian

AU - Popescu, Horia

AU - Sacchi, Maurizio

AU - Sardinha, Anna B.

AU - Sirotti, Fausto

AU - Zeitoun, Philippe

AU - Messerschmidt, Marc

AU - Turner, Joshua J.

AU - Schlotter, William F.

AU - Hellwig, Olav

AU - Mattana, Richard

AU - Jaouen, Nicolas

AU - Fortuna, Franck

AU - Acremann, Yves

AU - Gutt, Christian

AU - Dürr, Hermann A.

AU - Beaurepaire, Eric

AU - Boeglin, Christine

AU - Eisebitt, Stefan

AU - Grübel, Gerhard

AU - Lüning, Jan

AU - Stöhr, Joachim

AU - Scherz, Andreas O.

N1 - Funding Information: We would like to thank I. Ferrero for providing the dIrr data points included in Fig. 4. This work was supported by the Science and Technology Facilities Council [grant number ST/F001166/1 and RF040218], the European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013)/ERC Grant agreement 278594-GasAroundGalaxies, the National Science Foundation under Grant No. PHYS-1066293, the Interuniversity Attraction Poles Programme of the Belgian Science Policy Office [AP P7/08 CHARM] and the hospitality of the Aspen Center for Physics. MF and TS acknowledge the Marie-Curie ITN CosmoComp, and MF also acknowledges the ERC Advanced Grant programme Dustygal. CSF acknowledges an ERC Advanced Investigator Grant COSMIWAY. This work used the DiRAC Data Centric system at Durham University, operated by the Institute for Computational Cosmology on behalf of the STFC DiRAC HPC Facility (www.dirac.ac.uk), and resources provided by WestGrid (www.westgrid.ca) and Compute Canada/Calcul Canada (www.computecanada.ca). The DiRAC system is funded by BIS National E-infrastructure capital grant ST/K00042X/1, STFC capital grant ST/H008519/1, STFC DiRAC Operations grant ST/K003267/1 and Durham University. DiRAC is part of the National E-Infrastructure. Funding Information: We would like to thank I. Ferrero for providing the dIrr data points included in Fig. 4. This work was supported by the Science and Technology Facilities Council [grant number ST/F001166/1 and RF040218], the European Research Council under the European Union’s Seventh Framework Programme (FP7/2007-2013)/ERC Grant agreement 278594-GasAroundGalaxies, the National Science Foundation under Grant No. PHYS-1066293, the Interuniversity Attraction Poles Programme of the Belgian Science Policy Office [AP P7/08 CHARM] and the hospitality of the Aspen Center for Physics. MF and TS acknowledge the Marie-Curie ITN CosmoComp, and MF also acknowledges the ERC Advanced Grant programme Dustygal. CSF acknowledges an ERC Advanced Investigator Grant COSMIWAY. This work used the DiRAC Data Centric system at Durham University, operated by the Institute for Computational Cosmology on behalf of the STFC DiRAC HPC Facility (www.dirac.ac.uk), and resources provided by WestGrid (www.westgrid.ca) and Compute Canada/Calcul Canada (www.computecanada.ca). The DiRAC system is funded by BIS National E-infrastructure capital grant ST/K00042X/1, STFC capital grant ST/H008519/1, STFC DiRAC Operations grant ST/K003267/1 and Durham University. DiRAC is part of the National E-Infrastructure.

PY - 2012/6/27

Y1 - 2012/6/27

N2 - We present the first single-shot images of ferromagnetic, nanoscale spin order taken with femtosecond x-ray pulses. X-ray-induced electron and spin dynamics can be outrun with pulses shorter than 80 fs in the investigated fluence regime, and no permanent aftereffects in the samples are observed below a fluence of 25mJ/cm2. Employing resonant spatially muliplexed x-ray holography results in a low imaging threshold of 5mJ/cm2. Our results open new ways to combine ultrafast laser spectroscopy with sequential snapshot imaging on a single sample, generating a movie of excited state dynamics.

AB - We present the first single-shot images of ferromagnetic, nanoscale spin order taken with femtosecond x-ray pulses. X-ray-induced electron and spin dynamics can be outrun with pulses shorter than 80 fs in the investigated fluence regime, and no permanent aftereffects in the samples are observed below a fluence of 25mJ/cm2. Employing resonant spatially muliplexed x-ray holography results in a low imaging threshold of 5mJ/cm2. Our results open new ways to combine ultrafast laser spectroscopy with sequential snapshot imaging on a single sample, generating a movie of excited state dynamics.

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U2 - 10.1103/PhysRevLett.108.267403

DO - 10.1103/PhysRevLett.108.267403

M3 - Article

AN - SCOPUS:84862992483

SN - 0031-9007

VL - 108

JO - Physical Review Letters

JF - Physical Review Letters

IS - 26

M1 - 267403

ER -

Femtosecond single-shot imaging of nanoscale ferromagnetic order in co/pd multilayers using resonant x-ray holography

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