Abstract
The effect of α-particle irradiation on a NdFeAs(O,F) thin film has been investigated to determine how the introduction of defects affects basic superconducting properties, including the critical temperature T c and the upper critical field H c2, and properties more of interest for applications, like the critical current density J c and the related pinning landscape. The irradiation-induced suppression of the film T c is significantly smaller than on a similarly damaged single crystal. Moreover H c2 behaves differently, depending on the field orientation: for H//c the H c2 slope monotonically increases with increasing disorder, whereas for H//ab it remains constant at low dose and it increases only when the sample is highly disordered. This suggests that a much higher damage level is necessary to drive the NdFeAs(O,F) thin film into the dirty limit. Despite the increase in the low temperature H c2, the effects on the J c(H//c) performances are moderate in the measured temperature and field ranges, with a shifting of the pinning force maximum from 4.5 to 6 T after an irradiation of 2 1015 cm-2. On the contrary, J c(H//ab) is always suppressed. The analysis demonstrates that irradiation does introduce point defects (PD) acting as pinning centres proportionally to the irradiation fluence but also suppresses the effectiveness of c-axis correlated pinning present in the pristine sample. We estimate that significant performance improvements may be possible at high field or at temperatures below 10 K. The suppression of the J c(H//ab) performance is not related to a decrease of the J c anisotropy as found in other superconductors. Instead it is due to the presence of PD that decrease the efficiency of the ab-plane intrinsic pinning typical of materials with a layered structure.
Original language | English (US) |
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Article number | 034002 |
Journal | Superconductor Science and Technology |
Volume | 31 |
Issue number | 3 |
DOIs | |
State | Published - Feb 5 2018 |
Keywords
- critical current
- Fe-based superconductors
- irradiation, pinning properties
- NdFeAs(O,F)
ASJC Scopus subject areas
- Ceramics and Composites
- Condensed Matter Physics
- Metals and Alloys
- Electrical and Electronic Engineering
- Materials Chemistry