Diffractive electron imaging of nanoparticles on a substrate.

Research output: Contribution to journalArticle

28 Citations (Scopus)

Abstract

The observation of the detailed atomic arrangement within nanostructures has previously required the use of an electron microscope for imaging. The development of diffractive (lensless) imaging in X-ray science and electron microscopy using ab initio phase retrieval provides a promising tool for nanostructural characterization. We show that it is possible experimentally to reconstruct the atomic-resolution complex image (exit-face wavefunction) of a small particle lying on a thin carbon substrate from its electron microdiffraction pattern alone. We use a modified iterative charge-flipping algorithm and an estimate of the complex substrate image is subtracted at each iteration. The diffraction pattern is recorded using a parallel beam with a diameter of approximately 50 nm, illuminating a gold nanoparticle of approximately 13.6 nm diameter. Prior knowledge of the boundary of the object is not required. The method has the advantage that the reconstructed exit-face wavefunction is free of the aberrations of the objective lens normally used in the microscope, whereas resolution is limited only by thermal vibration and noise.

Original languageEnglish (US)
Pages (from-to)912-916
Number of pages5
JournalNature materials.
Volume4
Issue number12
StatePublished - Dec 2005

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Wave functions
Nanoparticles
Imaging techniques
nanoparticles
Electrons
Substrates
Aberrations
Gold
illuminating
Diffraction patterns
Electron microscopy
retrieval
iteration
aberration
Lenses
Nanostructures
electron microscopy
Microscopes
electrons
Electron microscopes

ASJC Scopus subject areas

  • Engineering(all)

Cite this

Diffractive electron imaging of nanoparticles on a substrate. / Wu, Jinsong; Weierstall, Uwe; Spence, John.

In: Nature materials., Vol. 4, No. 12, 12.2005, p. 912-916.

Research output: Contribution to journalArticle

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